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Continuous flow removal of acid fuchsine by dielectric barrier discharge plasma water bed enhanced by

Rusen Zhou, Renwu Zhou, Xianhui Zhang, Kateryna Bazaka, Kostya (Ken) Ostrikov

《化学科学与工程前沿（英文）》 2019年 第13卷 第2期   页码 340-349 doi: 10.1007/s11705-019-1798-z

摘要： Continuous processes which allow for large amount of wastewater to be treated to meet drainage standards while reducing treatment time and energy consumption are urgently needed. In this study, a dielectric barrier discharge plasma water bed system was designed and then coupled with granular activated carbon (GAC) adsorption to rapidly remove acid fuchsine (AF) with high efficiency. Effects of feeding gases, treatment time and initial concentration of AF on removal efficiency were investigated. Results showed that compared to the N and air plasmas treatments, O plasma processing was most effective for AF degradation due to the strong oxidation ability of generated activated species, especially the OH radicals. The addition of GAC significantly enhanced the removal efficiency of AF in aqueous solution and shorten the required time by 50%. The effect was attributed to the ability of porous carbon to trap and concentrate the dye, increasing the time dye molecules were exposed to the plasma treated solution, and to enhance the production of OH radicals on/in GAC to boost the degradation of dyes by plasma as well as in situ regenerate the exhausted GAC. The study offers a new opportunity for continuous effective remediation of wastewater contaminated with organic dyes using plasma technologies.

关键词： continuous removal     dye-containing wastewater     dielectric barrier discharge     plasma water bed     activated carbon adsorption    

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Abatement of mixed volatile organic compounds in a catalytic hybrid surface/packed-bed discharge plasma

Lianjie Guo, Nan Jiang, Jie Li, Kefeng Shang, Na Lu, Yan Wu

《环境科学与工程前沿（英文）》 2018年 第12卷 第2期 doi: 10.1007/s11783-018-1017-z

摘要： In this study, post plasma-catalysis degradation of mixed volatile organic compounds (benzene, toluene, and xylene) has been performed in a hybrid surface/packed-bed discharge plasma reactor with Ag-Ce/ g-Al O catalyst at room temperature. The effect of relative air humidity on mixed VOCs degradation has also been investigated in both plasma-only and PPC systems. In comparison to the plasma-only system, a significant improvement can be observed in the degradation performance of mixed VOCs in PPC system with Ag-Ce/ g-Al O catalyst. In PPC system, 68% benzene, 89% toluene, and 94% xylene were degraded at 800 J·L , respectively, which were 25%, 11%, and 9% higher than those in plasma-only system. This result can be attributed to the high catalytic activity of Ag-Ce/ g-Al O catalyst to effectively decompose O and lead to generating more reactive species which are capable of destructing the VOCs molecules completely. Moreover, the presence of Ag-Ce/ g-Al O catalyst in plasma significantly decreased the emission of discharge byproducts (NO and O ) and promoted the mineralization of mixed VOCs towards CO . Adding a small amount of water vapor into PPC system enhanced the degradation efficiencies of mixed VOCs, however, further increasing water vapor had a negative impact on the degradation efficiencies, which was primarily attributed to the quenching of energetic electrons by water vapor in plasma and the competitive adsorption of water vapor on the catalyst surface. Meanwhile, the catalysts before and after discharge were characterized by the Brunauer-Emment-Teller and X-ray photoelectron spectroscopy.

关键词： Mixed VOCs     HSPBD plasma reactor     Degradation     Catalyst     Relative humidity    

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From plasma to plasmonics: toward sustainable and clean water production through membranes

《化学科学与工程前沿（英文）》 2023年 第17卷 第12期   页码 1809-1836 doi: 10.1007/s11705-023-2339-3

摘要： The increasing demand for potable water is never-ending. Freshwater resources are scarce and stress is accumulating on other alternatives. Therefore, new technologies and novel optimization methods are developed for the existing processes. Membrane-based processes are among the most efficient methods for water treatment. Yet, membranes suffer from severe operational problems, namely fouling and temperature polarization. These effects can harm the membrane’s permeability, permeate recovery, and lifetime. To mitigate such effects, membranes can be treated through two techniques: plasma treatment (a surface modification technique), and treatment through the use of plasmonic materials (surface and bulk modification). This article showcases plasma- and plasmonic-based treatments in the context of water desalination/purification. It aims to offer a comprehensive review of the current developments in membrane-based water treatment technologies along with suggested directions to enhance its overall efficiency through careful selection of material and system design. Moreover, basic guidelines and strategies are outlined on the different membrane modification techniques to evaluate its prerequisites. Besides, we discuss the challenges and future developments about these membrane modification methods.

关键词： water treatment     membrane-based process     plasma treatment     plasma polymerization     plasmonic     light-to-heat conversion    

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Heat flux distribution on circulating fluidized bed boiler water wall

LU Junfu, YUE Guangxi, YANG Hairui, ZHANG Jiansheng, YU Long, ZHANG Man, YANG Zhongming

《能源前沿（英文）》 2008年 第2卷 第2期   页码 134-139 doi: 10.1007/s11708-008-0027-0

摘要： The future of circulating fluidized bed (CFB) combustion technology is in raising the steam parameters to supercritical levels. Understanding the heat flux distribution on the water wall is one of the most important issues in the design and operation of supercritical pressure CFB boilers. In the present paper, the finite element analysis (FEA) method is adopted to predict the heat transfer coefficient as well as the heat flux of the membrane wall and the results are validated by direct measurement of the temperature around the tube. Studies on the horizontal heat flux distribution were conducted in three CFB boilers with different furnace size, tube dimension and water temperature. The results are useful in supercritical pressure CFB boiler design.

关键词： horizontal     different furnace     temperature     FEA     measurement    

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Reduction of hexavalent chromium with scrap iron in a fixed bed reactor

Yin WANG, Xuejiang WANG, Xin WANG, Mian LIU, Siqing XIA, Daqiang YIN, Yalei ZHANG, Jianfu ZHAO

《环境科学与工程前沿（英文）》 2012年 第6卷 第6期   页码 761-769 doi: 10.1007/s11783-012-0413-z

摘要： The reduction of hexavalent chromium by scrap iron was investigated in continuous long-term fixed bed system. The effects of pH, empty bed contact time (EBCT), and initial Cr(VI) concentration on Cr(VI) reduction were studied. The results showed that the pH, EBCT, and initial Cr(VI) concentration significantly affected the reduction capacity of scrap iron. The reduction capacity of scrap iron were 4.56, 1.51, and 0.57 mg Cr(VI)·g Fe at pH 3, 5, and 7 (initial Cr(VI) concentration 4 mg·L , EBCT 2 min, and temperature 25°C), 0.51, 1.51, and 2.85 mg Cr(VI)·g Fe at EBCTs of 0.5, 2.0, and 6.0 min (initial Cr(VI) concentration 4 mg·L , pH 5, and temperature 25°C), and 2.99, 1.51, and 1.01 mg Cr(VI)·g Fe at influent concentrations of 1, 4, and 8 mg·L (EBCT 2 min, pH 5, and temperature 25°C), respectively. Fe(total) concentration in the column effluent continuously decreased in time, due to a decrease in time of the iron corrosion rate. The fixed bed reactor can be readily used for the treatment of drinking water containing low amounts of Cr(VI) ions, although the hardness and humic acid in water may shorten the lifetime of the reactor, the reduction capacity of scrap iron still achieved 1.98 mg Cr ·g Fe. Scanning electron microscope equipped with energy dispersion spectrometer and X-ray diffraction were conducted to examine the surface species of the scrap iron before and after its use. In addition to iron oxides and hydroxide species, iron-chromium complex was also observed on the reacted scrap iron.

关键词： hexavalent chromium     scrap iron     reduction capacity     drinking water    

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水平管道淤积断面紊流的速度分布研究

王冬梅,张士林

《中国工程科学》 2005年 第7卷 第2期   页码 66-68

摘要：

对固定床水平管道断面的紊流速度分布进行研究。将整个断面分为弓形圆弧断面和渗流断面。弓形圆弧断面的速度分布研究基于圆形断面管道紊流理论，并且结合一定的假设数值模拟弓形圆弧断面管道的紊流速度分布规律；渗流断面的速度分布研究基于渗流理论。通过一定的边界条件将两部分断面速度分布组合成整个断面的速度分布。大量的实验证明本研究方法及程序较好地模拟了此断面的紊流速度分布。

关键词： 弓形圆弧断面     固定床     紊流速度     零剪力点     水力坡度    

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Diagnostic evaluation of plasma aldosterone concentration to plasma renin activity ratio in primary aldosteronism

ZHANG Huilan, WANG Daowen

《医学前沿（英文）》 2008年 第2卷 第1期   页码 11-14 doi: 10.1007/s11684-008-0003-4

摘要： Using the plasma aldosterone concentration to plasma renin activity ratio (PAC/PRA ratio) as the screening test of choice for primary aldosteronism in hypertensive patients, we studied the clinical characteristics and the diagnostic value of PAC/PRA ratio in primary aldosteronism. The plasma aldosterone concentration (PAC) and plasma renin activity (PRA) levels were measured by radioimmunoassay in 902 hypertensive patients from out-patient clinics or hospitals. One hundred and twenty-six suspected primary aldosteronism patients whose PAC/PRA ratio was > 25 ng/dL/ng/mL/hr had a lamellar computed tomography (CT) scan in the adrenal gland and follow-up visits. The proportion of primary aldosteronism in hypertensive patients was 14% (126/902). There were 54 patients with unilateral or bilateral hyperplasia and 25 patients with adenoma according to the CT scan. 39% (49/126) of the patients with primary aldosteronism had hypokalemia. Twenty-five patients received surgical treatment. The efficacy and cure rates were 100% (25/25) and 48% (12/25), respectively. The effective rate of aldactone and the single-drug cure rate were 89% (48/54) and 24% (13/54), respectively. Primary aldosteronism affects over 10% of hypertensive patients in China. The PAC/PRA ratio can be considered as a routine screening test in hypertensives, especially resistant hypertensive patients and a high PAC/PRA ratio is an invaluable index in primary aldosteronism diagnosis.
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Important parameters in plasma jets for the production of RONS in liquids for plasma medicine: A brief

Anna Khlyustova, Cédric Labay, Zdenko Machala, Maria-Pau Ginebra, Cristina Canal

《化学科学与工程前沿（英文）》 2019年 第13卷 第2期   页码 238-252 doi: 10.1007/s11705-019-1801-8

摘要： Reactive oxygen and nitrogen species (RONS) are among the key factors in plasma medicine. They are generated by atmospheric plasmas in biological fluids, living tissues and in a variety of liquids. This ability of plasmas to create a delicate mix of RONS in liquids has been used to design remote or indirect treatments for oncological therapy by treating biological fluids by plasmas and putting them in contact with the tumour. Documented effects include selective cancer cell toxicity, even though the exact mechanisms involved are still under investigation. However, the “right” dose for suitable therapeutical activity is crucial and still under debate. The wide variety of plasma sources hampers comparisons. This review focuses on atmospheric pressure plasma jets as the most studied plasma devices in plasma medicine and compiles the conditions employed to generate RONS in relevant liquids and the concentration ranges obtained. The concentrations of H O , NO , NO and short-lived oxygen species are compared critically to provide a useful overview for the reader.

关键词： atmospheric plasma jets     liquids     ROS     RNS     plasma-dose    

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Kinetic Monte Carlo simulations of plasma-surface reactions on heterogeneous surfaces

Daniil Marinov

《化学科学与工程前沿（英文）》 2019年 第13卷 第4期   页码 815-822 doi: 10.1007/s11705-019-1837-9

摘要： Reactions of atoms and molecules on chamber walls in contact with low temperature plasmas are important in various technological applications. Plasma-surface interactions are complex and relatively poorly understood. Experiments performed over the last decade by several groups prove that interactions of reactive species with relevant plasma-facing materials are characterized by distributions of adsorption energy and reactivity. In this paper, we develop a kinetic Monte Carlo (KMC) model that can effectively handle chemical kinetics on such heterogenous surfaces. Using this model, we analyse published adsorption-desorption kinetics of chlorine molecules and recombination of oxygen atoms on rotating substrates as a test case for the KMC model.

关键词： plasma-surface interaction     kinetic Monte Carlo     plasma nano technology    

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Atomistic simulations of plasma catalytic processes

Erik C. Neyts

《化学科学与工程前沿（英文）》 2018年 第12卷 第1期   页码 145-154 doi: 10.1007/s11705-017-1674-7

摘要： There is currently a growing interest in the realisation and optimization of hybrid plasma/catalyst systems for a multitude of applications, ranging from nanotechnology to environmental chemistry. In spite of this interest, there is, however, a lack in fundamental understanding of the underlying processes in such systems. While a lot of experimental research is already being carried out to gain this understanding, only recently the first simulations have appeared in the literature. In this contribution, an overview is presented on atomic scale simulations of plasma catalytic processes as carried out in our group. In particular, this contribution focusses on plasma-assisted catalyzed carbon nanostructure growth, and plasma catalysis for greenhouse gas conversion. Attention is paid to what can routinely be done, and where challenges persist.

关键词： atomic scale simulation     plasma-catalyst    

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Plasma-catalysis: Is it just a question of scale?

J. Christopher Whitehead

《化学科学与工程前沿（英文）》 2019年 第13卷 第2期   页码 264-273 doi: 10.1007/s11705-019-1794-3

摘要： The issues of describing and understanding the changes in performance that result when a catalyst is placed into plasma are discussed. The different chemical and physical interactions that result and how their combination might produce beneficial results for the plasma-catalytic processing of different gas streams are outlined with particular emphasis being placed on the different range of spatial and temporal scales that must be considered both in experiment and modelling. The focus is on non-thermal plasma where the lack of thermal equilibrium creates a range of temperature scales that must be considered. This contributes in part to a wide range of inhomogeneity in different properties such as species concentrations and electric fields that must be determined experimentally by methods and be incorporated into modelling. It is concluded that plasma-catalysis is best regarded as conventional catalysis perturbed by the presence of a discharge, which modifies its operating conditions, properties and outcomes often in a very localised way. The sometimes used description “plasma-activated catalysis” is an apt one.

关键词： plasma catalysis     plasma-activated catalysis     non-thermal plasma     CO2 conversion    

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Restoration of hyper-eutrophic water with a modularized and air adjustable constructed submerged plantbed

Jinzhong LI, Xueju LI, Shujuan SUN, Xuegong LIU, Suiliang HUANG

《环境科学与工程前沿（英文）》 2011年 第5卷 第4期   页码 573-584 doi: 10.1007/s11783-011-0363-x

摘要： A modularized and air adjustable constructed submerged plant bed (CSPB) which can be used to restore the eutrophic water is introduced in this paper. This plant bed helps hydrophyte grow under poor conditions such as frequently changed water depth, impaired water transparency, algae bloom and substantial duckweed in summer, which are not naturally suitable for growing hydrophyte. This pilot study in Waihuan River of Tianjin, China, revealed that reduction of Chemical Oxygen Demand (COD), Total Nitrogen (TN) and Total Phosphorus (TP) by the use of CSPB could be reached 30%–35%, 35%–40%, 30%–40% respectively in the growing season (from March to October) and 5%–10%, 5%–15%, 7%–20% respectively in the winter (from November to February) when the detention time was 6 d. The relationships between the concentration of COD, TN, TP and the detention time fit the first-order kinetic equation well and the coefficients of determination ( ) were all above 0.9. The attenuation coefficients k of the kinetic equation were a function of the water temperature. When the water temperature was quite low or quite high, was not significantly changed with increasing or decreasing water temperature. While when the temperature was in a moderate range, an increase or decrease of water temperature would lead to a rapid increase or decrease in .

关键词： modularized and air adjustable constructed submerged plant bed     water purification     eco-restoration techniques     aquatic plants     eutrophication    

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Submerged arc plasma system combined with ozone oxidation for the treatment of wastewater containing

《环境科学与工程前沿（英文）》 2021年 第15卷 第5期 doi: 10.1007/s11783-020-1384-0

摘要：

• Submerged arc plasma was introduced in terms of wastewater treatment.

关键词： Thermal plasma     Submerged arc plasma     Wastewater     Ozone     Phenol     Highly energetic electron    

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Prediction of bed load sediments using different artificial neural network models

Reza ASHEGHI, Seyed Abbas HOSSEINI

《结构与土木工程前沿（英文）》 2020年 第14卷 第2期   页码 374-386 doi: 10.1007/s11709-019-0600-0

摘要： Modeling and prediction of bed loads is an important but difficult issue in river engineering. The introduced empirical equations due to restricted applicability even in similar conditions provide different accuracies with each other and measured data. In this paper, three different artificial neural networks (ANNs) including multilayer percepterons, radial based function (RBF), and generalized feed forward neural network using five dominant parameters of bed load transport formulas for the Main Fork Red River in Idaho-USA were developed. The optimum models were found through 102 data sets of flow discharge, flow velocity, water surface slopes, flow depth, and mean grain size. The deficiency of empirical equations for this river by conducted comparison between measured and predicted values was approved where the ANN models presented more consistence and closer estimation to observed data. The coefficient of determination between measured and predicted values for empirical equations varied from 0.10 to 0.21 against the 0.93 to 0.98 in ANN models. The accuracy performance of all models was evaluated and interpreted using different statistical error criteria, analytical graphs and confusion matrixes. Although the ANN models predicted compatible outputs but the RBF with 79% correct classification rate corresponding to 0.191 network error was outperform than others.

关键词： bed load prediction     artificial neural network     modeling     empirical equations    

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Liquefaction and impurity separation of oxygen-bearing coal-bed methane

Qiuying LI, Yonglin JU, Li WANG,

《能源前沿（英文）》 2010年 第4卷 第3期   页码 319-325 doi: 10.1007/s11708-010-0115-9

摘要： Coal-bed methane (CBM) is a type of clean energy. However, most oxygen-bearing CBM have not yet to be utilized due to limited techniques, and when utilized, the discharged gas leads to resource wastage and environment pollution. In this paper, a liquefaction process is proposed and designed for the specified oxygen-bearing CBM obtained from the Daqing Qingshen gas field. The distillation column is employed to separate the oxygen and nitrogen components present in the CBM. HYSYS software is adopted to simulate the process, and the results reveal that the energy consumption of the whole liquefaction process is low. Moreover, oxygen and nitrogen are nearly removed completely, achieving a high-purity liquefied natural gas product with a high methane recovery rate. The applicability and safety of the liquefaction process are also analyzed. The simulation results can offer references for the separation of the oxygen component from CBM.

关键词： coal bed methane     oxygen-bearing     liquefaction     distillation    

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标题 作者 时间 类型 操作

Continuous flow removal of acid fuchsine by dielectric barrier discharge plasma water bed enhanced by

Rusen Zhou, Renwu Zhou, Xianhui Zhang, Kateryna Bazaka, Kostya (Ken) Ostrikov

期刊论文

Abatement of mixed volatile organic compounds in a catalytic hybrid surface/packed-bed discharge plasma

Lianjie Guo, Nan Jiang, Jie Li, Kefeng Shang, Na Lu, Yan Wu

期刊论文

From plasma to plasmonics: toward sustainable and clean water production through membranes

期刊论文

Heat flux distribution on circulating fluidized bed boiler water wall

LU Junfu, YUE Guangxi, YANG Hairui, ZHANG Jiansheng, YU Long, ZHANG Man, YANG Zhongming

期刊论文

Reduction of hexavalent chromium with scrap iron in a fixed bed reactor

Yin WANG, Xuejiang WANG, Xin WANG, Mian LIU, Siqing XIA, Daqiang YIN, Yalei ZHANG, Jianfu ZHAO

期刊论文

水平管道淤积断面紊流的速度分布研究

王冬梅,张士林

期刊论文

Diagnostic evaluation of plasma aldosterone concentration to plasma renin activity ratio in primary aldosteronism

ZHANG Huilan, WANG Daowen

期刊论文

Important parameters in plasma jets for the production of RONS in liquids for plasma medicine: A brief

Anna Khlyustova, Cédric Labay, Zdenko Machala, Maria-Pau Ginebra, Cristina Canal

期刊论文

Kinetic Monte Carlo simulations of plasma-surface reactions on heterogeneous surfaces

Daniil Marinov

期刊论文

Atomistic simulations of plasma catalytic processes

Erik C. Neyts

期刊论文

Plasma-catalysis: Is it just a question of scale?

J. Christopher Whitehead

期刊论文

Restoration of hyper-eutrophic water with a modularized and air adjustable constructed submerged plantbed

Jinzhong LI, Xueju LI, Shujuan SUN, Xuegong LIU, Suiliang HUANG

期刊论文

Submerged arc plasma system combined with ozone oxidation for the treatment of wastewater containing

期刊论文

Prediction of bed load sediments using different artificial neural network models

Reza ASHEGHI, Seyed Abbas HOSSEINI

期刊论文

Liquefaction and impurity separation of oxygen-bearing coal-bed methane

Qiuying LI, Yonglin JU, Li WANG,

期刊论文